Sequential deposition route to efficient Sb2S3 solar cells

doi:10.1039/c8ta08296k

CORC > 合肥物质科学研究院 > 中国科学院合肥物质科学研究院 > 应用技术研究所

	Sequential deposition route to efficient Sb2S3 solar cells
	Zhang, Lijian 1; Wu, Chunyan 1; Liu, Weifeng 1; Yang, Shangfeng 1; Wang, Mingtai 2; Chen, Tao 1; Zhu, Changfei 1
刊名	JOURNAL OF MATERIALS CHEMISTRY A
	2018-11-21
卷号	6 期号:43 页码:21320-21326
ISSN号	2050-7488
DOI	10.1039/c8ta08296k
通讯作者	Chen, Tao(tchenmse@ustc.edu.cn) ; Zhu, Changfei(cfzhu@ustc.edu.cn)
英文摘要	We report a facile two-step sequential deposition method to prepare Sb2S3 thin films, where antimony acetate and thiourea are utilized as antimony and sulfur sources, respectively. The sequential deposition of two precursor materials followed by swift annealing at mild temperature leads to high-quality Sb2S3 films. The detailed reaction mechanism is revealed on the basis of structural and compositional analyses. By optimizing the concentration of thiourea and annealing temperature, uniform and flat Sb2S3 thin films are obtained with either sulfur-deficiency or sulfur richness. Finally, a planar heterojunction solar cell based on the as-prepared Sb2S3 film delivers a high power conversion efficiency of 5.69%, which is a top value for planar heterojunction Sb2S3 solar cells fabricated by a solution approach. This research provides a convenient and low-cost approach for the deposition of Sb2S3 films for efficient solar cell applications.
资助项目	Fundamental Research Funds for the Central Universities[WK2060140023] ; Fundamental Research Funds for the Central Universities[WK2060140022] ; Fundamental Research Funds for the Central Universities[CX3430000001] ; Fundamental Research Funds for the Central Universities[WK2060140024] ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology[2016FXZY003] ; Recruitment Program of Global Experts (National Natural Science Foundation of China)[GG2060140085]
WOS关键词	ATOMIC LAYER DEPOSITION ; THERMAL-DECOMPOSITION ; THIN-FILMS ; THIOUREA ; ABSORBER ; GROWTH
WOS研究方向	Chemistry ; Energy & Fuels ; Materials Science
语种	英语
出版者	ROYAL SOC CHEMISTRY
WOS记录号	WOS:000449701900007
资助机构	Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; 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Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China)
内容类型	期刊论文
源URL	[http://ir.hfcas.ac.cn:8080/handle/334002/34163]
专题	合肥物质科学研究院_应用技术研究所
通讯作者	Chen, Tao; Zhu, Changfei
作者单位	1.Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, 96 Jinzhai Rd, Hefei 230026, Anhui, Peoples R China 2.Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Hefei 230031, Anhui, Peoples R China
推荐引用方式 GB/T 7714	Zhang, Lijian,Wu, Chunyan,Liu, Weifeng,et al. Sequential deposition route to efficient Sb2S3 solar cells[J]. JOURNAL OF MATERIALS CHEMISTRY A,2018,6(43):21320-21326.
APA	Zhang, Lijian.,Wu, Chunyan.,Liu, Weifeng.,Yang, Shangfeng.,Wang, Mingtai.,...&Zhu, Changfei.(2018).Sequential deposition route to efficient Sb2S3 solar cells.JOURNAL OF MATERIALS CHEMISTRY A,6(43),21320-21326.
MLA	Zhang, Lijian,et al."Sequential deposition route to efficient Sb2S3 solar cells".JOURNAL OF MATERIALS CHEMISTRY A 6.43(2018):21320-21326.