Cu-2(oh)po4/reduced graphene oxide nanocomposites for enhanced photocatalytic degradation of 2,4-dichlorophenol under infrared light irradiation | |
Zhang, Chenyang1,2; Du, Zhen2; Zhou, Ruyi2; Xu, Peng4; Dong, Xinghua2,3; Fu, Yanyan6; Wang, Qing5; Su, Chunjian1; Yan, Liang2,3; Gu, Zhanjun2,3 | |
刊名 | Rsc advances |
2018 | |
卷号 | 8期号:7页码:3611-3618 |
ISSN号 | 2046-2069 |
DOI | 10.1039/c7ra12684k |
通讯作者 | Fu, yanyan(fuyy@mail.sim.ac.cn) ; Su, chunjian(suchunjian2008@163.com) ; Yan, liang(yanliang@ihep.ac.cn) ; Gu, zhanjun(zjgu@ihep.ac.cn) |
英文摘要 | Sparked by the growing environmental crises, photocatalytic degradation of chlorophenols with inexhaustible solar energy is expected to be converted into actual applications. here, we report the preparation of the nanocomposite of cu-2(oh)po4 and reduced graphene oxide (cu-2(oh)po4/rgo) through a one-step hydrothermal method and examined its infrared-light photocatalytic activity in the degradation of 2,4-dichlorophenol (2,4-dcp). as evidenced by the absorption spectra and the degradation of 2,4-dcp, cu-2(oh)po4/rgo exhibited enhanced infrared light-driven photocatalytic activity compared to pure cu-2(oh)po4 and was very stable even after repeated cycling. more importantly, the introduction of hydrogen peroxide (h2o2) could combine the photocatalytic and photo-fenton effects into one reaction system and maximize the infrared light photocatalytic efficiency. typically, the rate constant of cu-2(oh)po4/rgo and h2o2 was more than 6.25 times higher than that of only cu-2(oh)po4/rgo, and almost 10 times greater than the value for pure cu-2(oh)po4. further, a plausible mechanism for the enhanced photocatalytic properties of cu-2(oh)po4/rgo has been discussed. these findings may help the development of novel hybrid photocatalysts with enhanced infrared light photocatalytic activity for applications in the treatment of chlorophenol-contaminated wastewater. |
WOS关键词 | HYDROGEN-PEROXIDE ; CONTROLLED-RELEASE ; CHLOROPHENOLS ; PERFORMANCE ; COMPOSITES ; PESTICIDES ; SURFACE ; TIO2 ; 4-CHLOROPHENOL ; ADSORPTION |
WOS研究方向 | Chemistry |
WOS类目 | Chemistry, Multidisciplinary |
语种 | 英语 |
出版者 | ROYAL SOC CHEMISTRY |
WOS记录号 | WOS:000423348500030 |
内容类型 | 期刊论文 |
URI标识 | http://www.corc.org.cn/handle/1471x/2177915 |
专题 | 高能物理研究所 |
通讯作者 | Fu, Yanyan; Su, Chunjian; Yan, Liang; Gu, Zhanjun |
作者单位 | 1.Shandong Univ Sci & Technol, Coll Mech & Elect Engn, Qingdao 266590, Peoples R China 2.Chinese Acad Sci, Inst High Energy Phys, Key Lab Biomed Effects Nanomat & Nanosafety, Beijing 100049, Peoples R China 3.Univ Chinese Acad Sci, Beijing 101408, Peoples R China 4.Natl Ctr Nanoscience & Technol, Key Lab Standardizat & Measurement Nanotechnol, Beijing 100190, Peoples R China 5.Shandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R China 6.Chinese Acad Sci, Shanghai Inst Microsystem & Informat Technol, State Key Lab Transducer Technol, Changning Rd 865, Shanghai 200050, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Chenyang,Du, Zhen,Zhou, Ruyi,et al. Cu-2(oh)po4/reduced graphene oxide nanocomposites for enhanced photocatalytic degradation of 2,4-dichlorophenol under infrared light irradiation[J]. Rsc advances,2018,8(7):3611-3618. |
APA | Zhang, Chenyang.,Du, Zhen.,Zhou, Ruyi.,Xu, Peng.,Dong, Xinghua.,...&Gu, Zhanjun.(2018).Cu-2(oh)po4/reduced graphene oxide nanocomposites for enhanced photocatalytic degradation of 2,4-dichlorophenol under infrared light irradiation.Rsc advances,8(7),3611-3618. |
MLA | Zhang, Chenyang,et al."Cu-2(oh)po4/reduced graphene oxide nanocomposites for enhanced photocatalytic degradation of 2,4-dichlorophenol under infrared light irradiation".Rsc advances 8.7(2018):3611-3618. |
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