Catalytic reduction of low-concentration CO2 with water by Pt/Co@NC

doi:10.1016/j.jmst.2018.04.010

	Catalytic reduction of low-concentration CO2 with water by Pt/Co@NC
	Wang, Qianqian 1,2; Wang, Wenzhong 2; Zhang, Ling 2; Su, Yang 2; Wang, Kefu 2; Wu, Huixia 1
刊名	JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
	2018
卷号	34 期号:12 页码:2337
关键词	Carbon dioxide catalytic reduction Pt/Co@NC Low-concentration CO2 No sacrificial agent
ISSN号	1005-0302
DOI	10.1016/j.jmst.2018.04.010
英文摘要	The reduction of low-concentration carbon dioxide with water to organic fuels is still a huge challenge. In this study, we successfully designed the partially oxidized cobalt nanoparticles coated by the nitrogen-doped carbon layer (Co@NC) of 2-8 nm via a facile method and then interspersed with different amount of Pt nanoparticles. The Co@NC decorated with 1 wt% Pt exhibits the best ability for CO2 reduction to CH4 and a CH4 production rate of 14.4 mu mol.g(-1). h(-1) is achieved. It is worth noting that the system is carried out under low-concentration CO2 (400 ppm) circumstance without any sacrificial agent, which could be meaningful to the design of catalysts for atmospheric CO2 reduction. (C) 2018 Published by Elsevier Ltd on behalf of The editorial office of Journal of Materials Science & Technology.
学科主题	Materials Science, Multidisciplinary ; Metallurgy & Metallurgical Engineering
出版者	JOURNAL MATER SCI TECHNOL
WOS记录号	WOS:000443274500015
资助机构	This work was financially supported by the National Natural Science Foundation of China (Nos. 51772312 and 51472260), the Environmental Functional Materials Innovation Team of Ministry of Education (IRT_16R49), and the International Joint Laboratory on Resource Chemistry (IJLRC). ; This work was financially supported by the National Natural Science Foundation of China (Nos. 51772312 and 51472260), the Environmental Functional Materials Innovation Team of Ministry of Education (IRT_16R49), and the International Joint Laboratory on Resource Chemistry (IJLRC).
内容类型	期刊论文
源URL	[http://ir.sic.ac.cn/handle/331005/24625]
专题	中国科学院上海硅酸盐研究所
作者单位	1.Shanghai Normal Univ, Shanghai Key Lab Rare Earth Funct Mat, Key Lab Resource Chem, Minist Educ, Shanghai 200234, Peoples R China 2.Shanghai Normal Univ, Shanghai Municipal Educ Comm, Key Lab Mol Imaging Probes & Sensors, Shanghai 200234, Peoples R China 3.Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Super Fine, Shanghai 200050, Peoples R China
推荐引用方式 GB/T 7714	Wang, Qianqian,Wang, Wenzhong,Zhang, Ling,et al. Catalytic reduction of low-concentration CO2 with water by Pt/Co@NC[J]. JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,2018,34(12):2337, 2341.
APA	Wang, Qianqian,Wang, Wenzhong,Zhang, Ling,Su, Yang,Wang, Kefu,&Wu, Huixia.(2018).Catalytic reduction of low-concentration CO2 with water by Pt/Co@NC.JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,34(12),2337.
MLA	Wang, Qianqian,et al."Catalytic reduction of low-concentration CO2 with water by Pt/Co@NC".JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY 34.12(2018):2337.