Guiding growth orientation of two-dimensional Au nanocrystals with marine chitin nanofibrils for ultrasensitive and ultrafast sensing hybrids
Chen, Yijun1,2; Liu, Zhengqin2; Li, Mingjie1; Wu, Xiaochen1; You, Jun1; Li, Chaoxu1
刊名JOURNAL OF MATERIALS CHEMISTRY B
2017-12-28
卷号5期号:48页码:9502-9506
DOI10.1039/c7tb02792c
产权排序1
文献子类Article
英文摘要We demonstrate that marine chitin nanofibrils are able to modulate the growth direction of two-dimensional Au nanocrystals from nanoribbons, nanokites to nanosheets. The mechanism investigation reveals that deacetylation and exfoliation of chitin nanofibrils are essential to template directional growth of Au nanocrystals. The tight adhesion of chitin nanofibrils on the Au surface enables the design of functional hybrids as ultrafast and ultrasensitive responsive devices for humidity and pressure. Interestingly, the humidity responsive device shows an abrupt increase in resistance of up to 3 orders of magnitude with a tiny variation of relative humidity from 62% RH to 63% RH, and was capable of precisely sensing speech. As a conductive filler, only 0.09 vol% gold nanoribbons are able to append to tissue paper with a sheet resistance of up to 220 Omega sq(-1), which can be used as a frequently-used pressure-sensing device. These sensing hybrids are highly promising in smart clothing and electronic skins.
WOS关键词PERCOLATION-THRESHOLD ; GOLD NANOBELTS ; HUMIDITY SENSOR ; NANOCOMPOSITES ; NANOSHEETS ; WHISKERS
WOS研究方向Materials Science
语种英语
WOS记录号WOS:000418072200007
资助机构National Natural Science Foundation of China(21474125 ; Chinese "1000 Youth Talent Program'' ; Shandong "Taishan Youth Scholar Program'' ; Natural Science Foundation of Shandong Province(JQ201609) ; Shandong Collaborative Innovation Centre for Marine Biomass Fiber Materials and Textiles ; 51603224)
内容类型期刊论文
源URL[http://ir.qibebt.ac.cn/handle/337004/9819]  
专题青岛生物能源与过程研究所_仿生智能材料团队
通讯作者Liu, Zhengqin; You, Jun; Li, Chaoxu
作者单位1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, CAS Key Lab Biobased Mat, Qingdao 266101, Peoples R China
2.Qingdao Univ, Coll Text & Clothing, Qingdao 266071, Peoples R China
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Chen, Yijun,Liu, Zhengqin,Li, Mingjie,et al. Guiding growth orientation of two-dimensional Au nanocrystals with marine chitin nanofibrils for ultrasensitive and ultrafast sensing hybrids[J]. JOURNAL OF MATERIALS CHEMISTRY B,2017,5(48):9502-9506.
APA Chen, Yijun,Liu, Zhengqin,Li, Mingjie,Wu, Xiaochen,You, Jun,&Li, Chaoxu.(2017).Guiding growth orientation of two-dimensional Au nanocrystals with marine chitin nanofibrils for ultrasensitive and ultrafast sensing hybrids.JOURNAL OF MATERIALS CHEMISTRY B,5(48),9502-9506.
MLA Chen, Yijun,et al."Guiding growth orientation of two-dimensional Au nanocrystals with marine chitin nanofibrils for ultrasensitive and ultrafast sensing hybrids".JOURNAL OF MATERIALS CHEMISTRY B 5.48(2017):9502-9506.
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