Characterization of polychlorinated biphenyl congeners in surface sediments of the Changjiang Estuary and adjacent shelf by high-resolution sampling and high-resolution mass spectrometry

doi:10.1016/j.marpolbul.2017.07.036

CORC > 青岛生物能源与过程研究所 > 中国科学院青岛生物能源与过程研究所 > 材料生物技术研究中心

	Characterization of polychlorinated biphenyl congeners in surface sediments of the Changjiang Estuary and adjacent shelf by high-resolution sampling and high-resolution mass spectrometry
	Liu, Aifeng 1; Wang, Yawei 2; Xian, Mo 1; Zhao, Zongshan 1; Zhao, Bin 3; Wang, Jinpeng 3; Yao, Peng 3
刊名	MARINE POLLUTION BULLETIN
	2017-11-15
卷号	124 期号:1 页码:496-501
关键词	Polychlorinated Biphenyl Sediment Changjiang Estuary Distribution High-resolution
DOI	10.1016/j.marpolbul.2017.07.036
文献子类	Article
英文摘要	Due to limited samples and low-resolution analysis, conflicting findings on major polychlorinated biphenyl (PCB) congeners and their origins remain in the East China Sea (ECS). Based on high-resolution sampling and high-resolution mass spectrometry analysis, 72 surface sediment samples from the Changjiang Estuary and adjacent ECS shelf were determined to characterize 39 PCB congeners. PCBs (Sigma(39)PCBs) ranged from 0.003 to 16.18 ng/g dw, presenting a decreasing seaward trend. Tri-, tetra- and penta-CBs were the main components, accounting for > 64% of Sigma(39)PCBs in most samples. Tetra-CBs were the dominant congeners, corresponding to results of sediments from Changjiang middle reach and soils from Changjiang Delta. Comparison between PCBs and sediment properties indicated there may be a deposition boundary of 30 degrees N. In the north, the spatial distribution of PCBs is controlled by Changjiang input and hydrodynamic conditions, while in the south closely related to combination of local source and riverine input.
WOS关键词	EAST CHINA SEA ; YANGTZE-RIVER DELTA ; ORGANOCHLORINE-PESTICIDES ; ORGANIC POLLUTANTS ; CONTINENTAL-SHELF ; RISK-ASSESSMENT ; PCB CONGENERS ; DEGRADATION ; DECHLORINATION ; DISTRIBUTIONS
WOS研究方向	Environmental Sciences & Ecology ; Marine & Freshwater Biology
语种	英语
WOS记录号	WOS:000415391200067
资助机构	China Postdoctoral Science Foundation(2016M602210) ; National Natural Science Foundation of China(21407086 ; State Key Laboratory of Environmental Chemistry and Ecotoxicology Open Fund(KF2016-12) ; 21477138 ; 41676063 ; 41521064)
内容类型	期刊论文
源URL	[http://ir.qibebt.ac.cn/handle/337004/9690]
专题	青岛生物能源与过程研究所_材料生物技术研究中心
作者单位	1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, CAS Key Lab Biobased Mat, Qingdao 266101, Peoples R China 2.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, POB 2871, Beijing 100085, Peoples R China 3.Ocean Univ China, Minist Educ, Key Lab Marine Chem Theory & Technol, Qingdao 266100, Peoples R China
推荐引用方式 GB/T 7714	Liu, Aifeng,Wang, Yawei,Xian, Mo,et al. Characterization of polychlorinated biphenyl congeners in surface sediments of the Changjiang Estuary and adjacent shelf by high-resolution sampling and high-resolution mass spectrometry[J]. MARINE POLLUTION BULLETIN,2017,124(1):496-501.
APA	Liu, Aifeng.,Wang, Yawei.,Xian, Mo.,Zhao, Zongshan.,Zhao, Bin.,...&Yao, Peng.(2017).Characterization of polychlorinated biphenyl congeners in surface sediments of the Changjiang Estuary and adjacent shelf by high-resolution sampling and high-resolution mass spectrometry.MARINE POLLUTION BULLETIN,124(1),496-501.
MLA	Liu, Aifeng,et al."Characterization of polychlorinated biphenyl congeners in surface sediments of the Changjiang Estuary and adjacent shelf by high-resolution sampling and high-resolution mass spectrometry".MARINE POLLUTION BULLETIN 124.1(2017):496-501.