Enhanced Photophosphorylation of a Chloroplast-Entrapping Long-Lived Photoacid
Xu, Youqian1,2; Fei, Jinbo1; Li, Guangle1,2; Yuan, Tingting1,2; Li, Yue1,2; Wang, Chenlei1,2; Li, Xianbao1,2; Li, Junbai1,2
刊名ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
2017-10-09
卷号56期号:42页码:12903-12907
关键词Chloroplasts Photoacids Photophosphorylation Photosynthesis
英文摘要Enhancing solar energy conversion efficiency is very important for developing renewable energy, protecting the environment, and producing agricultural products. Efficient enhancement of photophosphorylation is demonstrated by coupling artificial photoacid generators (PAGs) with chloroplasts. The encapsulation of small molecular long-lived PAGs in the thylakoid lumen is improved greatly by ultrasonication. Under visible-light irradiation, a fast intramolecular photoreaction of the PAG occurs and produces many protons, remarkably enhancing the proton gradient insitu. Consequently, compared to pure chloroplasts, the assembled natural-artificial hybrid demonstrates approximately 3.9 times greater adenosine triphosphate (ATP) production. This work will provide new opportunities for constructing enhanced solar energy conversion systems.
语种英语
内容类型期刊论文
源URL[http://ir.iccas.ac.cn/handle/121111/41237]  
专题化学研究所_胶体、界面与化学热力学实验室
作者单位1.Chinese Acad Sci, Inst Chem, Key Lab Colloid Interface & Chem Thermodynam, BNLMS CAS, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Xu, Youqian,Fei, Jinbo,Li, Guangle,et al. Enhanced Photophosphorylation of a Chloroplast-Entrapping Long-Lived Photoacid[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2017,56(42):12903-12907.
APA Xu, Youqian.,Fei, Jinbo.,Li, Guangle.,Yuan, Tingting.,Li, Yue.,...&Li, Junbai.(2017).Enhanced Photophosphorylation of a Chloroplast-Entrapping Long-Lived Photoacid.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,56(42),12903-12907.
MLA Xu, Youqian,et al."Enhanced Photophosphorylation of a Chloroplast-Entrapping Long-Lived Photoacid".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 56.42(2017):12903-12907.
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