Three-dimensional porous vanadium nitride nanoribbon aerogels as Pt-free counter electrode for high-performance dye-sensitized solar cells | |
Wang, Guiqiang1; Hou, Shuo1; Yan, Chao1; Lin, Yuan2; Liu, Shaomin3 | |
刊名 | CHEMICAL ENGINEERING JOURNAL |
2017-08-15 | |
卷号 | 322页码:611-617 |
关键词 | Porous Vanadium Nitride Nanoribbon Electrocatalytic Activity Aerogels Counter Electrode Dye-sensitized Solar Cells |
英文摘要 | Three-dimensional (3D) porous vanadium nitride nanoribbon aerogels (PVNNRAs) are prepared by hydrothermal synthesis and subsequent nitridation in ammonia/argon atmosphere and investigated as Pt-free counter electrode in dye-sensitized solar cells (DSCs). 3D porous nanoribbon aerogel can simultaneously offer more electrocatalytic active sites, a fast electron-transport pathway, and a favorable electrolyte diffusion channel, which endows the PVNNRA electrode with high electrocatalytic activity for the reduction of I-3(-). Under full-sun illumination (AM 1.5, 100 mW cm(-2)), the DSC fabricated with PVNNRA counter electrode achieves a conversion efficiency of 7.05%, which is comparable to that of DSCs fabricated with Pt counter electrode. In addition, the PVNNRA electrode exhibits good stability in redox electrolyte. Thus, 3D PVNNRAs can be considered as a cost-effective alternative to Pt as the counter electrode of DSCs. (C) 2017 Elsevier B.V. All rights reserved. |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.iccas.ac.cn/handle/121111/38410] |
专题 | 化学研究所_光化学实验室 |
作者单位 | 1.Bohai Univ, Sch New Energy, Jinzhou 121013, Peoples R China 2.Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China 3.Curtin Univ, Dept Chem Engn, Perth, WA 6845, Australia |
推荐引用方式 GB/T 7714 | Wang, Guiqiang,Hou, Shuo,Yan, Chao,et al. Three-dimensional porous vanadium nitride nanoribbon aerogels as Pt-free counter electrode for high-performance dye-sensitized solar cells[J]. CHEMICAL ENGINEERING JOURNAL,2017,322:611-617. |
APA | Wang, Guiqiang,Hou, Shuo,Yan, Chao,Lin, Yuan,&Liu, Shaomin.(2017).Three-dimensional porous vanadium nitride nanoribbon aerogels as Pt-free counter electrode for high-performance dye-sensitized solar cells.CHEMICAL ENGINEERING JOURNAL,322,611-617. |
MLA | Wang, Guiqiang,et al."Three-dimensional porous vanadium nitride nanoribbon aerogels as Pt-free counter electrode for high-performance dye-sensitized solar cells".CHEMICAL ENGINEERING JOURNAL 322(2017):611-617. |
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