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Two-Photon Absorption of Cationic Conjugated Polyelectrolytes: Effects of Aggregation and Application to 2-Photon-Sensitized Fluorescence from Green Fluorescent Protein
Wang, Shanshan1,2; Li, Zhiliang1,2; Liu, Xinglei4; Phan, Samantha1,2; Lv, Fengting5; Belfield, Kevin D.4; Wang, Shu5; Schanze, Kirk S.1,2,3
刊名CHEMISTRY OF MATERIALS
2017-04-11
卷号29期号:7页码:3295-3303
英文摘要Two cationic conjugated polyelectrolytes (CPEs) based on poly(phenylene ethynylene) are found to exhibit efficient 2-photon excited fluorescence. In particular,. the CPE aggregates display enhanced 2-photon absorption compared to the nonaggregated states. The CPEs are used as 2-photon absorption sensitizers to harvest light and amplify the fluorescence from green fluorescent protein (GFP) through Forster resonance energy transfer. Considerably enhanced GFP fluorescence under near-infrared 2-photon excitation is demonstrated both in solution and in HeLa cells. The results suggest applications in 2-photon fluorescence imaging of cells, tissues, and organs of living animals expressing GFP.
语种英语
内容类型期刊论文
源URL[http://ir.iccas.ac.cn/handle/121111/38337]  
专题化学研究所_有机固体实验室
作者单位1.Univ Florida, Dept Chem, Gainesville, FL 32611 USA
2.Univ Florida, Ctr Macromol Sci & Engn, Gainesville, FL 32611 USA
3.Univ Texas San Antonio, Dept Chem, One UTSA Circle, San Antonio, TX 78249 USA
4.New Jersey Inst Technol, Dept Chem & Environm Sci, Newark, NJ 07102 USA
5.Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Key Lab Organ Solids, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Wang, Shanshan,Li, Zhiliang,Liu, Xinglei,et al. Two-Photon Absorption of Cationic Conjugated Polyelectrolytes: Effects of Aggregation and Application to 2-Photon-Sensitized Fluorescence from Green Fluorescent Protein[J]. CHEMISTRY OF MATERIALS,2017,29(7):3295-3303.
APA Wang, Shanshan.,Li, Zhiliang.,Liu, Xinglei.,Phan, Samantha.,Lv, Fengting.,...&Schanze, Kirk S..(2017).Two-Photon Absorption of Cationic Conjugated Polyelectrolytes: Effects of Aggregation and Application to 2-Photon-Sensitized Fluorescence from Green Fluorescent Protein.CHEMISTRY OF MATERIALS,29(7),3295-3303.
MLA Wang, Shanshan,et al."Two-Photon Absorption of Cationic Conjugated Polyelectrolytes: Effects of Aggregation and Application to 2-Photon-Sensitized Fluorescence from Green Fluorescent Protein".CHEMISTRY OF MATERIALS 29.7(2017):3295-3303.
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