Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression | |
Iwamoto, M; Wu, CX; Zhong-Can, OY; Iwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan. | |
刊名 | CHEMICAL PHYSICS LETTERS |
2000 | |
卷号 | 325期号:41035页码:545-551 |
关键词 | Circular-dichroism Spectroscopy Optical 2nd-harmonic Generation 2nd Harmonic-generation Molecular-orientation Rotational Averages Surface Films |
ISSN号 | 0009-2614 |
英文摘要 | The complete expression for the macroscopic second-order susceptibility (SOS) tensor chi((2)) for a monolayer with C-infinity symmetry at the air-liquid interface is derived as functions of the molecular SOS tensor alpha((2)) and the orientational order parameters. The chiral (non-chiral) terms of chi((2)) distinguished by their association with even (odd) order parameters, by which a second-harmonic generation (SHG) circular-dichroism effect can be better understood. An SHG experiment of a 4-cyano-4'-5-alkyl-biphenyl monolayer on an air-water interface by monolayer compression is also discussed. (C) 2000 Elsevier Science B.V. All rights reserved. |
学科主题 | Physics |
URL标识 | 查看原文 |
WOS记录号 | WOS:000088612600011 |
公开日期 | 2012-08-29 |
内容类型 | 期刊论文 |
源URL | [http://ir.itp.ac.cn/handle/311006/12921] |
专题 | 理论物理研究所_理论物理所1978-2010年知识产出 |
通讯作者 | Iwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan. |
推荐引用方式 GB/T 7714 | Iwamoto, M,Wu, CX,Zhong-Can, OY,et al. Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression[J]. CHEMICAL PHYSICS LETTERS,2000,325(41035):545-551. |
APA | Iwamoto, M,Wu, CX,Zhong-Can, OY,&Iwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan..(2000).Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression.CHEMICAL PHYSICS LETTERS,325(41035),545-551. |
MLA | Iwamoto, M,et al."Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression".CHEMICAL PHYSICS LETTERS 325.41035(2000):545-551. |
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