Mass Spectral Analysis of the Aged 1,3,5-Trimethylbenzene Secondary Organic Aerosol in the Presence of Ammonium Sulfate Seeds

doi:10.15244/pjoes/66768

CORC > 合肥物质科学研究院 > 中国科学院合肥物质科学研究院 > 中科院安徽光学精密机械研究所

	Mass Spectral Analysis of the Aged 1,3,5-Trimethylbenzene Secondary Organic Aerosol in the Presence of Ammonium Sulfate Seeds
	Huang, Mingqiang 1,2; Xu, Jun 1; Cai, Shunyou 1; Liu, Xingqiang 2; Hui, Changjin 3; Gu, Xuejun 3; Fang, Li3 ; Zhang, Weijun 3
刊名	POLISH JOURNAL OF ENVIRONMENTAL STUDIES
	2017
卷号	26 期号:4 页码:1531-1537
关键词	Ammonium Sulfate 1 Secondary Organic Aerosol 3 Laser Time-of-flight Mass Spectrometer 5-trimethylbenzene Aging Mechanisms
DOI	10.15244/pjoes/66768
文献子类	Article
英文摘要	The ammonium sulfate ((NH4)(2)SO4) seed aerosols commonly found in the Chinese urban atmosphere could affect the formation and aging of secondary organic aerosols (SOA). Aging of aromatic SOA is performed using UV-irradiation of 1,3,5-trimethylbenzene (135-TMB)/CH3ONO/NO/air mixtures with high concentrations (similar to 100 mu g/m(3)) of (NH4)(2)SO4 seeds in the laboratory chamber in this study. The particulate products of SOA were measured using an aerosol laser time-of-flight mass spectrometer (ALTOFMS) in real-time, and fuzzy c-means (FCM) was applied to the mass spectra organic species for clusters. Experimental results indicated that methylglyxoal, 2-methyl-4-oxo-2-pentenal, 4-methyl-IH-imidazole, 4-methyl-imidazole-2-acetaldehyde, and other imidazole derivative compounds are the principal products in the aged particles. Imidazole compounds that can absorb solar radiation effectively were newly detected in the aged 135-TMB SOA with high concentrations of (NH4)(2)SO4 seed aerosols. These would provide new information for discussing the 135-TMB SOA aging mechanism.
WOS关键词	BROWN CARBON ; GAS-PHASE ; PARTICLES ; PHOTOOXIDATION ; GERMINATION ; PRODUCTS ; CHAMBER ; IMPACT ; IDENTIFICATION ; SPECTROMETER
WOS研究方向	Environmental Sciences & Ecology
语种	英语
WOS记录号	WOS:000408078000011
资助机构	National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; National Natural Science Foundation of China(41575118 ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Outstanding Youth Science Foundation of Fujian Province of China(2015J06009) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; Natural Science Foundation of Fujian Province of China(2015J05028) ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 41305109 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 21502086 ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126) ; 41575126)
内容类型	期刊论文
源URL	[http://ir.hfcas.ac.cn:8080/handle/334002/33640]
专题	合肥物质科学研究院_中科院安徽光学精密机械研究所
作者单位	1.Minnan Normal Univ, Coll Chem & Environm, Fujian Prov Key Lab Modern Analyt Sci & Separat T, Zhangzhou 363000, Peoples R China 2.Xiamen Univ, Dept Environm Sci & Engn, Tan Kah Kee Coll, Zhangzhou 363105, Peoples R China 3.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Lab Atmospher Physicochem, Hefei 230031, Anhui, Peoples R China
推荐引用方式 GB/T 7714	Huang, Mingqiang,Xu, Jun,Cai, Shunyou,et al. Mass Spectral Analysis of the Aged 1,3,5-Trimethylbenzene Secondary Organic Aerosol in the Presence of Ammonium Sulfate Seeds[J]. POLISH JOURNAL OF ENVIRONMENTAL STUDIES,2017,26(4):1531-1537.
APA	Huang, Mingqiang.,Xu, Jun.,Cai, Shunyou.,Liu, Xingqiang.,Hui, Changjin.,...&Zhang, Weijun.(2017).Mass Spectral Analysis of the Aged 1,3,5-Trimethylbenzene Secondary Organic Aerosol in the Presence of Ammonium Sulfate Seeds.POLISH JOURNAL OF ENVIRONMENTAL STUDIES,26(4),1531-1537.
MLA	Huang, Mingqiang,et al."Mass Spectral Analysis of the Aged 1,3,5-Trimethylbenzene Secondary Organic Aerosol in the Presence of Ammonium Sulfate Seeds".POLISH JOURNAL OF ENVIRONMENTAL STUDIES 26.4(2017):1531-1537.