Fabrication and photoelectrochemical properties of ZnS/Au/TiO2 nanotube array films | |
Zhu, Yan-Feng ; Zhang, Juan ; Xu, Lu ; Guo, Ya ; Wang, Xiao-Ping ; Du, Rong-Gui ; Lin, Chang-Jian ; Du RG(杜荣归) ; Lin CJ(林昌健) | |
刊名 | http://dx.doi.org/10.1039/c3cp43572e |
2013 | |
关键词 | SENSITIZED SOLAR-CELLS LIGHT PHOTOCATALYTIC ACTIVITY VISIBLE-LIGHT TIO2 NANOTUBES GOLD NANOPARTICLES TITANIUM-DIOXIDE DOPED TIO2 AU NANOPARTICLES FERMI-LEVEL NANOCOMPOSITES |
英文摘要 | National Natural Science Foundation of China [21173177, 21073151, 21021002]; A highly ordered TiO2 nanotube array film was fabricated by an anodic oxidation method. The film was modified by Au nanoparticles (NPs) formed by a deposition-precipitation technique and was covered with a thin ZnS shell prepared by a successive ionic layer adsorption and reaction (SILAR) method. The photoelectrochemical properties of the prepared ZnS/Au/TiO2 composite film were evaluated by incident photon-to-current conversion efficiency (IPCE), and photopotential and electrochemical impedance spectroscopy (EIS) measurements under white light illumination. The results indicated that the Au NPs could expand the light sensitivity range of the film and suppress the electron-hole recombination, and the ZnS shell could inhibit the leakage of photogenerated electrons from the surface of Au NPs to the ZnS/electrolyte interface. When the 403 stainless steel in a 0.5 M NaCl solution was coupled to the ZnS/Au/TiO2 nanotube film photoanode under illumination, its potential decreased by 400 mV, showing that the composite film had a better photocathodic protection effect on the steel than that of a pure TiO2 nanotube film. |
语种 | 英语 |
出版者 | ROYAL SOC CHEMISTRY |
内容类型 | 期刊论文 |
源URL | [http://dspace.xmu.edu.cn/handle/2288/88819] |
专题 | 化学化工-已发表论文 |
推荐引用方式 GB/T 7714 | Zhu, Yan-Feng,Zhang, Juan,Xu, Lu,et al. Fabrication and photoelectrochemical properties of ZnS/Au/TiO2 nanotube array films[J]. http://dx.doi.org/10.1039/c3cp43572e,2013. |
APA | Zhu, Yan-Feng.,Zhang, Juan.,Xu, Lu.,Guo, Ya.,Wang, Xiao-Ping.,...&林昌健.(2013).Fabrication and photoelectrochemical properties of ZnS/Au/TiO2 nanotube array films.http://dx.doi.org/10.1039/c3cp43572e. |
MLA | Zhu, Yan-Feng,et al."Fabrication and photoelectrochemical properties of ZnS/Au/TiO2 nanotube array films".http://dx.doi.org/10.1039/c3cp43572e (2013). |
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