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	Effect of high concentrations of inorganic seed aerosols on secondary organic aerosol formation in the m-xylene/NOx photooxidation system
	Lu, Zifeng ; Hao, Jiming ; Takekawa, Hideto ; Hu, Lanhua ; Li, Junhua
	2010-10-12 ; 2010-10-12
关键词	Secondary organic aerosol Aerosol yield Calcium sulfate Calcium nitrate Ammonium sulfate AMMONIUM-SULFATE AEROSOL ATMOSPHERIC AEROSOL AROMATIC-HYDROCARBONS ALPHA-PINENE TOLUENE OXIDATION IMPACT PM2.5 WATER MASS Environmental Sciences Meteorology & Atmospheric Sciences
中文摘要	High concentrations (>15 mu m(3) cm (3)) of CaSO4, Ca(NO3)(2), (NH4)(2)SO4 were selected as surrogates of dry neutral, aqueous neutral and dry acidic inorganic seed aerosols, respectively, to study the effects of inorganic seeds on secondary organic aerosol (SOA) formation in irradiated m-xylene/NOx photooxidation systems. The results indicate that neither ozone formation nor SOA formation is significantly affected by the presence of neutral aerosols (both dry CaSO4 and aqueous Ca(NO3)(2)), even at elevated concentrations. The presence of high concentrations of (NH4)(2)SO4 aerosols (dry acidic) has no obvious effect on ozone formation, but it does enhance SOA generation and increase SOA yields. In addition, the effect of dry (NH4)(2)SO4 on SOA yield is found to be positively Correlated with the (NH4)(2)SO4 surface concentration, and the effect is pronounced only when the Surface concentration reaches a threshold value. Further, it is proposed that the SOA generation enhancement is achieved by particle-phase heterogeneous reactions induced and catalyzed by the acidity of dry (NH4)(2)SO4 seed aerosols. (C) 2008 Elsevier Ltd. All rights reserved.
语种	英语 ; 英语
出版者	PERGAMON-ELSEVIER SCIENCE LTD ; OXFORD ; THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
内容类型	期刊论文
源URL	[http://hdl.handle.net/123456789/79862]
专题	清华大学
推荐引用方式 GB/T 7714	Lu, Zifeng,Hao, Jiming,Takekawa, Hideto,et al. Effect of high concentrations of inorganic seed aerosols on secondary organic aerosol formation in the m-xylene/NOx photooxidation system[J],2010, 2010.
APA	Lu, Zifeng,Hao, Jiming,Takekawa, Hideto,Hu, Lanhua,&Li, Junhua.(2010).Effect of high concentrations of inorganic seed aerosols on secondary organic aerosol formation in the m-xylene/NOx photooxidation system..
MLA	Lu, Zifeng,et al."Effect of high concentrations of inorganic seed aerosols on secondary organic aerosol formation in the m-xylene/NOx photooxidation system".(2010).

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