Functionalized graphene/Fe3O4 supported AuPt alloy as a magnetic, stable and recyclable catalyst for a catalytic reduction reaction

	Functionalized graphene/Fe3O4 supported AuPt alloy as a magnetic, stable and recyclable catalyst for a catalytic reduction reaction
	Gu,Wenling; Deng,XI; Jia,Xiaofang; Li,Jing; Wang,Erkang
刊名	journal of materials chemistry a
	2015
卷号	3 期号:16 页码:8793-8799
关键词	NOBLE-METAL NANOPARTICLES CORE-SHELL NANOPARTICLES GOLD NANOPARTICLES HIGHLY EFFICIENT FACILE SYNTHESIS COMPOSITE FE3O4/GRAPHENE NANOMATERIALS MICROSPHERES NANOSHEETS
通讯作者	wang,ek
英文摘要	herein, branched poly-(ethylenimine) functionalized graphene/iron oxide hybrid (termed as bgns/fe3o4) was chosen as an efficient support material to load aupt alloy nanoparticles for constructing a multifunctional nanocatalyst via a simple and controlled self-assembly approach. bgns/fe3o4 as a nanocarrier made the aupt alloy nanoparticles uniformly distributed on the surface of bgns/fe3o4. the obtained multifunctional nanocatalyst was characterized by high-resolution transmission electron microscopy (hrtem), energy dispersive x-ray (edx) spectroscopy, uv-vis spectroscopy and x-ray photoelectron spectroscopy (xps). the nanocatalyst exhibited favorable water solubility, excellent dispersion, good stability, superparamagnetism and particularly high catalytic activity for reducing 4-nitrophenol (4-np). furthermore, by tuning the composition of the nanoalloy nanoparticles of the multifunctional nanocatalyst, a normalized rate constant of about 17.99 mg(-1) s(-1) was achieved, which was superior to most of the au or pt based nanocatalysts reported in recent years. in addition, it was proved that the magnetic fe3o4 nanoparticles not only ensured the reuse of the nanocatalyst, but also significantly improved the catalytic activity. thanks to the favorable catalytic activity, the obtained multifunctional nanocatalyst may hold great potential for various catalytic processes.
收录类别	SCI
语种	英语
公开日期	2016-05-03
内容类型	期刊论文
源URL	[http://ir.ciac.jl.cn/handle/322003/64639]
专题	长春应用化学研究所_长春应用化学研究所知识产出_期刊论文
推荐引用方式 GB/T 7714	Gu,Wenling,Deng,XI,Jia,Xiaofang,et al. Functionalized graphene/Fe3O4 supported AuPt alloy as a magnetic, stable and recyclable catalyst for a catalytic reduction reaction[J]. journal of materials chemistry a,2015,3(16):8793-8799.
APA	Gu,Wenling,Deng,XI,Jia,Xiaofang,Li,Jing,&Wang,Erkang.(2015).Functionalized graphene/Fe3O4 supported AuPt alloy as a magnetic, stable and recyclable catalyst for a catalytic reduction reaction.journal of materials chemistry a,3(16),8793-8799.
MLA	Gu,Wenling,et al."Functionalized graphene/Fe3O4 supported AuPt alloy as a magnetic, stable and recyclable catalyst for a catalytic reduction reaction".journal of materials chemistry a 3.16(2015):8793-8799.